吕功煊,田彬.溴染料敏化担载Pt石墨烯催化可见光制氢、氘和氦[J].分子催化,2017,31(2):101-104
溴染料敏化担载Pt石墨烯催化可见光制氢、氘和氦
Formation of Deuterium and Helium during Photocatalytic Hydrogen Generation from Water Catalyzed by Pt-Graphene Sensitized with Br-dye under Visible Light Irradiation
投稿时间:2017-03-25  修订日期:2017-04-10
DOI:
中文关键词:  光催化还原质子  生成氘和氦  可见光辐照
英文关键词:photocatalytic reduction of proton  formation of deuterium and helium  visible light irradiation
基金项目:
作者单位
吕功煊 中国科学院兰州化学物理研究所 羰基合成与选择氧化国家重点实验室, 甘肃 兰州 730000 
田彬 中国科学院兰州化学物理研究所 羰基合成与选择氧化国家重点实验室, 甘肃 兰州 730000
中国科学院大学, 北京 100049 
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中文摘要:
      3He是理想的核聚变燃料,但是地球上3He的储量十分有限,大约只有500 kg.我们报道了在可见光光照条件下,溴染料敏化担载Pt石墨烯催化水还原为氢气过程中伴生少量氘和氦的实验现象.结果表明在温和条件下自水中的质子生产氘和氦的是可能的.
英文摘要:
      3He is a perfect fuel for nuclear fusion, however, the amount of 3He on the earth is very limited, only around 500 kg. Here, we report that small amount of deuterium and helium can be produced during photocatalytic hydrogen evolution from water catalyzed by Pt-graphene sensitized with Br-dye under visible light irradiation. This work raises a mild route to generate deuterium (D2) and helium (He) from proton in the water under very mild conditions.
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